Pressure-induced charge-transfer and structural transition in hexagonal multiferroic HoMnO3

التفاصيل البيبلوغرافية
العنوان: Pressure-induced charge-transfer and structural transition in hexagonal multiferroic HoMnO3
المؤلفون: Ottesen, Martin, Ehrenreich-Petersen, Emma, Kronbo, Camilla Hjort, Baudelet, François, Nataf, Lucie, Kantor, Innokenty, Jørgensen, Mads Ry Vogel, Bremholm, Martin
المصدر: Physical Review B. 107(13)
مصطلحات موضوعية: Naturvetenskap, Fysik, Den kondenserade materiens fysik, Natural Sciences, Physical Sciences, Condensed Matter Physics
الوصف: The structural properties of the hexagonal multiferroic h-HoMnO3 under high pressure have been explored using synchrotron x-ray diffraction and x-ray absorption spectroscopy in diamond anvil cells. The structure was found to undergo a pressure-induced phase transition at ∼24 GPa to a rhombohedrally distorted superstructure, which is isostructural to the oxygen-loaded h-RMnO3+δ (R=Y,Dy,Ho,Er; δ≈0.28) phases found in the same systems. The driving force behind the phase transition is the highly compressible ab plane which facilitates a gradual charge disproportionation of Mn(III) with pressure. We speculate this stabilizes the spin-liquid phase due to ferromagnetic coupling between neighboring Mn(II)/Mn(IV) and Mn(III). In addition, we demonstrate that the structural behavior is highly susceptible to nonhydrostatic conditions and the choice of pressure medium should be carefully made.
URL الوصول: https://lup.lub.lu.se/record/4a0b6d4a-e5d6-4a1f-82c2-e2fcdfb6e7d9
http://dx.doi.org/10.1103/PhysRevB.107.134115
قاعدة البيانات: SwePub
الوصف
تدمد:24699950
DOI:10.1103/PhysRevB.107.134115