Electronic Resource
Evaluation of Sputtering Processes in Strontium Iridate Thin Films
| العنوان: | Evaluation of Sputtering Processes in Strontium Iridate Thin Films |
|---|---|
| المؤلفون: | Ministerio de Ciencia e Innovación (España), Agencia Estatal de Investigación (España), University of Belgrade, European Commission, Fuentes, Víctor, Balcells, Lluis, Konstantinović, Z., Martínez, Benjamín, Pomar, Alberto |
| بيانات النشر: | Multidisciplinary Digital Publishing Institute 2024-02-01 |
| نوع الوثيقة: | Electronic Resource |
| مستخلص: | The growth of epitaxial thin films from the Ruddlesden–Popper series of strontium iridates by magnetron sputtering is analyzed. It was found that, even using a non-stoichiometric target, the films formed under various conditions were consistently of the perovskite-like n = ∞ SrIrO3 phase, with no evidence of other RP series phases. A detailed inspection of the temperature–oxygen phase diagram underscored that kinetics mechanisms prevail over thermodynamics considerations. The analysis of the angular distribution of sputtered iridium and strontium species indicated clearly different spatial distribution patterns. Additionally, significant backsputtering was detected at elevated temperatures. Thus, it is assumed that the interplay between these two kinetic phenomena is at the origin of the preferential nucleation of the SrIrO3 phase. In addition, strategies for controlling cation stoichiometry off-axis have also been explored. Finally, the long-term stability of the films has been demonstrated. |
| مصطلحات الفهرس: | Spin–orbit coupling, Epitaxial thin films, Complex oxides, Growth mechanisms, Magnetron sputtering, artículo |
| URL: | Publisher's version Sí info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-128410OB-I00/ES/INTERCONVERSION ESPIN-CARGA EN HETEROESTRUCTURAS DE OXIDOS PARA DISPOSITIVOS SOT info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/CEX2019-000917-S info:eu-repo/grantAgreement/EC/H2020/101007417 |
| الاتاحة: | Open access content. Open access content https://creativecommons.org/licenses/by/4.0 openAccess |
| ملاحظة: | English |
| Other Numbers: | CTK oai:digital.csic.es:10261/345218 Nanomaterials 14(3): 242 (2024) CEX2019-000917-S 10.3390/nano14030242 2079-4991 1431960423 |
| المصدر المساهم: | CSIC From OAIster®, provided by the OCLC Cooperative. |
| رقم الانضمام: | edsoai.on1431960423 |
| قاعدة البيانات: | OAIster |
| الوصف غير متاح. |