Electronic Resource

Ultrathin Light-Emitting Diodes with External Efficiency over 26% Based on Resurfaced Perovskite Nanocrystals

التفاصيل البيبلوغرافية
العنوان: Ultrathin Light-Emitting Diodes with External Efficiency over 26% Based on Resurfaced Perovskite Nanocrystals
المؤلفون: Wan, Q, Zheng, W, Zou, C, Carulli, F, Zhang, C, Song, H, Liu, M, Zhang, Q, Lin, L, Kong, L, Li, L, Brovelli, S, Qun Wan, Weilin Zheng, Chen Zou, Francesco Carulli, Congyang Zhang, Haili Song, Mingming Liu, Qinggang Zhang, Lih Y. Lin, Long Kong, Liang Li, Sergio Brovelli
بيانات النشر: American Chemical Society country:US 2023
نوع الوثيقة: Electronic Resource
مستخلص: Light-emitting diodes based on perovskite nanocrystals (PNCs-LEDs) have gained great interest for next-generation display and lighting technologies prized for their color purity, high brightness, and luminous efficiency which approach the intrinsic limit imposed by light extraction from the device structure. Although the time is ripe for the development of effective light outcoupling strategies to further boost the device performance, this technologically relevant aspect of PNC-LEDs is still without a definitive solution. Here, following theoretical guidelines and without the integration of complex photonic structures, we realize stable PNC-LEDs with external quantum efficiency (EQE) as high as 26.7%. Key to such performance is channeling the recombination zone in PNC emissive layers as thin as 10 nm, which we achieve by finely balancing charge transport using CsPbBr3 PNCs resurfaced with a nickel oxide layer. The ultrathin approach is general and, in principle, applicable to other perovskite nanostructures for fabricating highly efficient, color-tunable transparent LEDs.
مصطلحات الفهرس: Light-emitting diodes, Perovskite nanocrystals, Resurfacing, Otucoupling, info:eu-repo/semantics/article
URL: https://hdl.handle.net/10281/400923
info:eu-repo/semantics/altIdentifier/wos/WOS:000916931000001
volume:8
issue:2
firstpage:927
lastpage:934
numberofpages:8
journal:ACS ENERGY LETTERS
الاتاحة: Open access content. Open access content
info:eu-repo/semantics/openAccess
ملاحظة: ELETTRONICO
English
Other Numbers: ITBAO oai:boa.unimib.it:10281/400923
10.1021/acsenergylett.2c02802
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85146183146
1376721875
المصدر المساهم: BICOCCA OPEN ARCH
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رقم الانضمام: edsoai.on1376721875
قاعدة البيانات: OAIster