Electronic Resource

Determination of Silica and Germania Film Network Structures on Ru(0001) at the Atomic Scale

التفاصيل البيبلوغرافية
العنوان: Determination of Silica and Germania Film Network Structures on Ru(0001) at the Atomic Scale
المؤلفون: Lewandowski, A, Schlexer, P, Tosoni, S, Gura, L, Marschalik, P, Buchner, C, Burrall, H, Burson, K, Schneider, W, Pacchioni, G, Heyde, M, Lewandowski A. L., Schlexer P., Tosoni S., Gura L., Marschalik P., Buchner C., Burrall H., Burson K. M., Schneider W. -D., Pacchioni G., Heyde M.
بيانات النشر: American Chemical Society 2019
نوع الوثيقة: Electronic Resource
مستخلص: The detailed structure of silica and germania films supported on Ru(0001) metal substrates are compared to each other. Surface science techniques together with density functional theory calculations have been used to gain insights into the atomic arrangement of these prominent glass-forming materials. The monolayer films of these materials both show predominantly crystalline hexagonal lattices with characteristic domain boundary structures. For the germania monolayer films a large variety of ring elements within domain boundaries have been observed. Density functional calculations predict stronger interaction with the metal substrate for bilayer germania as compared to bilayer silica films. Scanning tunneling microscopy images with atomically resolved structural features have given access to silica and germania bilayer film structures. Both bilayer films form characteristic amorphous ring structures. However, the germania bilayer films appear to be more corrugated, pointing to a stronger interaction with the metal support thus giving rise to slightly different connectivity rules.
مصطلحات الفهرس: thin films, info:eu-repo/semantics/article
URL: http://hdl.handle.net/10281/260108
http://pubs.acs.org/journal/jpccck
info:eu-repo/semantics/altIdentifier/wos/WOS:000463844500038
volume:123
issue:13
firstpage:7889
lastpage:7897
numberofpages:9
journal:JOURNAL OF PHYSICAL CHEMISTRY. C
الاتاحة: Open access content. Open access content
ملاحظة: English
Other Numbers: ITBAO oai:boa.unimib.it:10281/260108
10.1021/acs.jpcc.8b07110
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85055160551
1308932237
المصدر المساهم: BICOCCA OPEN ARCH
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رقم الانضمام: edsoai.on1308932237
قاعدة البيانات: OAIster