Academic Journal

Structural involvement in the melting of the charge density wave in 1T-TiSe_{2}

التفاصيل البيبلوغرافية
العنوان: Structural involvement in the melting of the charge density wave in 1T-TiSe_{2}
المؤلفون: Max Burian, Michael Porer, Jose R. L. Mardegan, Vincent Esposito, Sergii Parchenko, Bulat Burganov, Namrata Gurung, Mahesh Ramakrishnan, Valerio Scagnoli, Hiroki Ueda, Sonia Francoual, Federica Fabrizi, Yoshikazu Tanaka, Tadashi Togashi, Yuya Kubota, Makina Yabashi, Kai Rossnagel, Steven L. Johnson, Urs Staub
المصدر: Physical Review Research, Vol 3, Iss 1, p 013128 (2021)
بيانات النشر: American Physical Society, 2021.
سنة النشر: 2021
المجموعة: LCC:Physics
مصطلحات موضوعية: Physics, QC1-999
الوصف: In this work, we use ultrafast pump-probe nonresonant and resonant x-ray diffraction to track the periodic lattice distortion and the electronic charge density wave in 1T-TiSe_{2} upon optical excitation. We observe a fluence regime in which the periodic lattice deformation is strongly suppressed but the charge density wave related Se 4p orbital order remains mostly intact. Complete melting of both structural and electronic order occurs four to five times faster than expected from a purely electronic charge-screening process, strongly suggesting a structurally assisted weakening of excitonic correlations. Our experimental data provide insight on the intricate coupling between structural and electronic order in stabilizing the periodic-lattice-distortion/charge-density-wave state in 1T-TiSe_{2}. The results further show that electron-phonon coupling can lead to different, energy dependent phase-transition pathways in condensed matter systems, opening different possibilities in the conception of nonequilibrium phenomena at the ultrafast scale.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 2643-1564
Relation: https://doaj.org/toc/2643-1564
DOI: 10.1103/PhysRevResearch.3.013128
URL الوصول: https://doaj.org/article/c5b299ac6f5e4d869f9838f8c7dff006
رقم الانضمام: edsdoj.5b299ac6f5e4d869f9838f8c7dff006
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:26431564
DOI:10.1103/PhysRevResearch.3.013128