Academic Journal

Observation of Thermally Induced Piezomagnetic Switching in Cu2OSeO3 Polymorph Synthesized under High‐Pressure

التفاصيل البيبلوغرافية
العنوان: Observation of Thermally Induced Piezomagnetic Switching in Cu2OSeO3 Polymorph Synthesized under High‐Pressure
المؤلفون: Hung‐Cheng Wu, Takuya Aoyama, Daisuke Morikawa, Daisuke Okuyama, Kazuhiro Nawa, Wei‐Tin Chen, Chan‐Hung Lu, Tsung‐Wen Yen, Shin‐Ming Huang, Stuart Calder, Shuki Torii, Kenya Ohgushi, Masami Terauchi, Taku J. Sato
المصدر: Advanced Physics Research, Vol 3, Iss 11, Pp n/a-n/a (2024)
بيانات النشر: Wiley-VCH, 2024.
سنة النشر: 2024
المجموعة: LCC:Physics
مصطلحات موضوعية: high‐pressure synthesis, neutron diffraction, piezomagnetic, structural distortion, uniaxial‐pressure, Physics, QC1-999
الوصف: Abstract A polymorph of Cu2OSeO3 with the distorted kagome lattice is successfully obtained using the high‐pressure synthesis technique (Cu2OSeO3‐HP). The structural analysis using X‐ray and neutron powder diffraction suggests that the tetrahedral Cu2+ clusters [similar to those in Cu2OSeO3 ambient‐pressure phase (Cu2OSeO3‐AP)] exist in Cu2OSeO3‐HP but with three symmetry inequivalent sites. No structural change is observed between 1.5 K and the room temperature. The complex magnetic H‐T phase diagram is established based on the temperature‐ and field‐dependent magnetization data, indicating two distinct antiferromagnetic phases at low and intermediate temperatures, in addition to the higher‐temperature spin‐glass‐like phase. The low temperature phase is identified by neutron powder diffraction refinements as a canted noncollinear antiferromagnetic order with a weak ferromagnetic component along the b‐axis. Size of the refined ordered moment is ≈1.00(4) µB in Cu2OSeO3‐HP, indicating a large enhancement compared to that of Cu2OSeO3‐AP (≈0.61 µB). By applying a uniaxial stress, finite enhancement of weak ferromagnetic component in the noncollinear antiferromagnetic phase in Cu2OSeO3‐HP is observed, which is the clear evidence of the piezomagnetic effect. Interestingly, the sign of the induced magnetization changes on heating from the low‐temperature to the intermediate‐temperature phases, indicating a novel piezomagnetic switching effect in this compound.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 2751-1200
Relation: https://doaj.org/toc/2751-1200
DOI: 10.1002/apxr.202400054
URL الوصول: https://doaj.org/article/077d5e262d194b6989bff0127abec57c
رقم الانضمام: edsdoj.077d5e262d194b6989bff0127abec57c
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:27511200
DOI:10.1002/apxr.202400054