التفاصيل البيبلوغرافية
| العنوان: |
Two-Dimensional Layered Co(OH) 2 /g‑C 3 N 4 /Ni(OH) 2 Ternary Nanocomposites for Enhanced Visible-Light Photocatalytic H 2 ‑Production Activity |
| المؤلفون: |
Jun Zhang (48506), Shuai Shao (1415941), Desen Zhou (10977205), Tingmin Di (10977208), Tielin Wang (2085421) |
| سنة النشر: |
2021 |
| المجموعة: |
Smithsonian Institution: Digital Repository |
| مصطلحات موضوعية: |
Biotechnology, Biological Sciences not elsewhere classified, 2 D ternary heterostructure nanocom., Ni, sample, Co, photocatalytic performance, photocatalytic H 2 production, g-C 3 N 4, contact |
| الوصف: |
Two-dimensional (2D) layered nanocomposite provides a surface-to-surface heterojunction, which is an effective way to improve the photocatalytic performance because larger contact areas can promote the separation rate of interfacial charge carriers. In this study, Co(OH) 2 /g-C 3 N 4 /Ni(OH) 2 2D layered photocatalysts have been successfully synthesized through a simple precipitation–hydrothermal method. The composite achieves a high H 2 -production rate of 899 μmol·h –1 ·g –1 , which exceeds the rate of samples only coupled with Co(OH) 2 and Ni(OH) 2 by 4.0 and 1.9 times, respectively. In addition, the activity is even higher than that of the optimized Pt-g-C 3 N 4 sample (1 wt. % Pt–C). The characterization results reveal the close contact of g-C 3 N 4 and Ni/Co hydroxides, and such a face-to-face contact can greatly improve the interfacial charge-transfer rate, resulting in a high photocatalytic performance. This work demonstrates a simple way to enhance the photocatalytic H 2 production of g-C 3 N 4 under the cooperative effect of Co(OH) 2 and Ni(OH) 2 and provides novel insights into constructing other 2D ternary heterostructure nanocomposites. |
| نوع الوثيقة: |
article in journal/newspaper |
| اللغة: |
unknown |
| Relation: |
https://figshare.com/articles/journal_contribution/Two-Dimensional_Layered_Co_OH_sub_2_sub_g_C_sub_3_sub_N_sub_4_sub_Ni_OH_sub_2_sub_Ternary_Nanocomposites_for_Enhanced_Visible-Light_Photocatalytic_H_sub_2_sub_Production_Activity/14788864 |
| DOI: |
10.1021/acsaem.1c01198.s001 |
| الاتاحة: |
https://doi.org/10.1021/acsaem.1c01198.s001 |
| Rights: |
CC BY-NC 4.0 |
| رقم الانضمام: |
edsbas.EFBAC7E4 |
| قاعدة البيانات: |
BASE |