Academic Journal
Early stage ettringite and monosulfoaluminate carbonation investigated by in situ Raman spectroscopy coupled with principal component analysis
| العنوان: | Early stage ettringite and monosulfoaluminate carbonation investigated by in situ Raman spectroscopy coupled with principal component analysis |
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| المؤلفون: | Brahim, Mohamed-Nadjib, Mechling, Jean-Michel, Janvier-Badosa, Sarah, Marchetti, Mario |
| المساهمون: | Institut Jean Lamour (IJL), Institut de Chimie - CNRS Chimie (INC-CNRS)-Université de Lorraine (UL)-Centre National de la Recherche Scientifique (CNRS), Formulation, Microstructure, Modélisation et Durabilité des Matériaux de Construction (MAST-FM2D ), Université Gustave Eiffel |
| المصدر: | ISSN: 2352-4928 ; Materials Today Communications ; https://univ-eiffel.hal.science/hal-04019304 ; Materials Today Communications, 2023, 35, pp.105539. ⟨10.1016/j.mtcomm.2023.105539⟩. |
| بيانات النشر: | HAL CCSD Elsevier |
| سنة النشر: | 2023 |
| المجموعة: | Université de Lorraine: HAL |
| مصطلحات موضوعية: | Materials Today Communications Carbonation Raman spectroscopy principal component analysis ettringite monosulfoaluminate, Carbonation, Raman spectroscopy, principal component analysis, ettringite, monosulfoaluminate, [SPI]Engineering Sciences [physics] |
| الوصف: | International audience ; This study investigates the early stages of monosulfoaluminate and ettringite carbonation using nondestructive in situ Raman spectroscopy monitoring. Coupling this technique with Principal Components Analysis enables relevant information to be extracted from spectral data such as anaccurate identification of the beginning of the reaction and of specific chemical phases. These two hydrates and some of their carbonation products can be well detected using this vibrational spectroscopy technique. Experiments were conducted on two pastes of hydrated yeelimite, in thepresence and in the absence of gypsum respectively, during their carbonation. The results confirmed the detection of the beginning of the carbonation and allowed us to identify some consumed and formed chemical phases in the early stages of the reaction. These outcomes of in situ Ramanspectroscopy monitoring study on cementitious phases could help understand the early chemical modifications occurring in complex environments such as cement pastes. |
| نوع الوثيقة: | article in journal/newspaper |
| اللغة: | English |
| Relation: | hal-04019304; https://univ-eiffel.hal.science/hal-04019304; https://univ-eiffel.hal.science/hal-04019304/document; https://univ-eiffel.hal.science/hal-04019304/file/2023-Materials_Today_Communications_Brahim_Mechling_Janvier-Badosa_Marchetti_preprint.pdf |
| DOI: | 10.1016/j.mtcomm.2023.105539 |
| الاتاحة: | https://univ-eiffel.hal.science/hal-04019304 https://univ-eiffel.hal.science/hal-04019304/document https://univ-eiffel.hal.science/hal-04019304/file/2023-Materials_Today_Communications_Brahim_Mechling_Janvier-Badosa_Marchetti_preprint.pdf https://doi.org/10.1016/j.mtcomm.2023.105539 |
| Rights: | info:eu-repo/semantics/OpenAccess |
| رقم الانضمام: | edsbas.EFA254BB |
| قاعدة البيانات: | BASE |
| DOI: | 10.1016/j.mtcomm.2023.105539 |
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