Academic Journal
Grafting of Poly(ionic liquid) Brushes through Fe 0 ‑Mediated Surface-Initiated Atom Transfer Radical Polymerization for Marine Antifouling
| العنوان: | Grafting of Poly(ionic liquid) Brushes through Fe 0 ‑Mediated Surface-Initiated Atom Transfer Radical Polymerization for Marine Antifouling |
|---|---|
| المؤلفون: | Daheng Wu, Jianing Wang, Xiaodong Yin, Runxiang Tan, Tao Zhang |
| سنة النشر: | 2024 |
| مصطلحات موضوعية: | Biophysics, Microbiology, Biotechnology, Immunology, Inorganic Chemistry, Plant Biology, Virology, Environmental Sciences not elsewhere classified, Chemical Sciences not elsewhere classified, Physical Sciences not elsewhere classified, sophisticated operation process, research provided pathways, poor polymerization efficiency, escherichia coli <, bacillus subtilis <, attracted considerable attention, 98 nm h, marine antifouling surface, 0 , marine antifouling applications, marine antifouling, 24 h, widespread fields, unparalleled speed, opposite plates, monomer solution, low attachment, ionic liquid, gradient thickness, efficiently synthesized |
| الوصف: | Surface-tethered poly(ionic liquid) brushes have attracted considerable attention in widespread fields, from bioengineering to marine antifouling. However, their applications have been constrained due to the poor polymerization efficiency and sophisticated operation process. In this work, we efficiently synthesized the poly(ionic liquid) brushes with unparalleled speed (up to 98 nm h –1 ) through Fe 0 -mediated surface-initiated atom transfer radical polymerization (Fe 0 SI-ATRP) while consuming only microliter of monomer solution under ambient conditions. We also demonstrated that poly(ionic liquid) brushes with gradient thickness and wettability were easily accessible by regulating the distance between the opposite plates of Fe 0 SI-ATRP. Moreover, the resultant poly(ionic liquid) brushes presented excellent antibacterial activities against Escherichia coli (99.2%) and Bacillus subtilis (88.1%) after 24 h and low attachment for proteins and marine algae (≤5%) for over 2 weeks. This research provided pathways to the facile and controllable fabrication of poly(ionic liquid) materials for marine antifouling applications. |
| نوع الوثيقة: | article in journal/newspaper |
| اللغة: | unknown |
| Relation: | https://figshare.com/articles/journal_contribution/Grafting_of_Poly_ionic_liquid_Brushes_through_Fe_sup_0_sup_Mediated_Surface-Initiated_Atom_Transfer_Radical_Polymerization_for_Marine_Antifouling/25343631 |
| DOI: | 10.1021/acs.langmuir.3c03852.s001 |
| الاتاحة: | https://doi.org/10.1021/acs.langmuir.3c03852.s001 https://figshare.com/articles/journal_contribution/Grafting_of_Poly_ionic_liquid_Brushes_through_Fe_sup_0_sup_Mediated_Surface-Initiated_Atom_Transfer_Radical_Polymerization_for_Marine_Antifouling/25343631 |
| Rights: | CC BY-NC 4.0 |
| رقم الانضمام: | edsbas.E3FBEA27 |
| قاعدة البيانات: | BASE |
| DOI: | 10.1021/acs.langmuir.3c03852.s001 |
|---|