التفاصيل البيبلوغرافية
العنوان: |
Collective Plasmon Coupling in Gold Nanoparticle Clusters for Highly Efficient Photothermal Therapy |
المؤلفون: |
Jinxing Chen (551698), Mingfu Gong (4032368), Yulong Fan (8820494), Ji Feng (1511020), Lili Han (1426681), Huolin L. Xin (1315002), Muhan Cao (2891723), Qiao Zhang (138583), Dong Zhang (73558), Dangyuan Lei (6311753), Yadong Yin (1437601) |
سنة النشر: |
2022 |
المجموعة: |
Smithsonian Institution: Digital Repository |
مصطلحات موضوعية: |
Biophysics, Medicine, Pharmacology, Biotechnology, Ecology, Infectious Diseases, Space Science, Biological Sciences not elsewhere classified, Chemical Sciences not elsewhere classified, Physical Sciences not elsewhere classified, wave electrodynamic simulations, plasmonic nanoparticle clusters, effective medium approximation, confined seeded growth, optimized growth conditions, highly efficient ptas, prepare various pncs, gold nanoparticle clusters, unity absorption efficiency, collective plasmon coupling, collective plasmon, absorption efficiency, optimized pncs, strong absorption, ptas ), nanoscale ptas, ∼ 84, work demonstrates, vivo <, universal strategy |
الوصف: |
Plasmonic nanomaterials with strong absorption at near-infrared frequencies are promising photothermal therapy agents (PTAs). The pursuit of high photothermal conversion efficiency has been the central focus of this research field. Here, we report the development of plasmonic nanoparticle clusters (PNCs) as highly efficient PTAs and provide a semiquantitative approach for calculating their resonant frequency and absorption efficiency by combining the effective medium approximation (EMA) theory and full-wave electrodynamic simulations. Guided by the theoretical prediction, we further develop a universal strategy of space-confined seeded growth to prepare various PNCs. Under optimized growth conditions, we achieve a record photothermal conversion efficiency of up to ∼84% for gold-based PNCs, which is attributed to the collective plasmon-coupling-induced near-unity absorption efficiency. We further demonstrate the extraordinary photothermal therapy performance of the optimized PNCs in in vivo application. Our work demonstrates the high feasibility and efficacy of PNCs as nanoscale PTAs. |
نوع الوثيقة: |
article in journal/newspaper |
اللغة: |
unknown |
Relation: |
https://figshare.com/articles/journal_contribution/Collective_Plasmon_Coupling_in_Gold_Nanoparticle_Clusters_for_Highly_Efficient_Photothermal_Therapy/18320072 |
DOI: |
10.1021/acsnano.1c08485.s001 |
الاتاحة: |
https://doi.org/10.1021/acsnano.1c08485.s001 |
Rights: |
CC BY-NC 4.0 |
رقم الانضمام: |
edsbas.C2E41A04 |
قاعدة البيانات: |
BASE |