Academic Journal
Step by Step Construction of Multifunctional Hollow Double Shell MNPs@MOF as a Powerful Tandem/Cascade Catalyst
| العنوان: | Step by Step Construction of Multifunctional Hollow Double Shell MNPs@MOF as a Powerful Tandem/Cascade Catalyst |
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| المؤلفون: | Shi, Shunli, Yu, Ying, Zhang, Bingzhen, Zhong, Yicheng, Wang, Lei, Wang, Shuhua, Ding, Shunmin, Chen, Chao |
| المساهمون: | National Natural Science Foundation of China, Natural Science Foundation of Jiangxi Province |
| المصدر: | Frontiers in Chemistry ; volume 9 ; ISSN 2296-2646 |
| بيانات النشر: | Frontiers Media SA |
| سنة النشر: | 2021 |
| المجموعة: | Frontiers (Publisher - via CrossRef) |
| الوصف: | The development of efficient heterogeneous catalysts for one-pot tandem/cascade synthesis of imines remains meaningful and challenging. Herein, we constructed an Au/MOF catalyst featured hollow and double MOF shell nanostructure. Owing to its structural merits and acid-basic nature, the as-synthesized Void|(Au)ZIF-8|ZIF-8 catalyst exhibited an enhanced synergistically catalytic performance for tandem catalytic synthesis of imines from benzyl alcohol and aniline under air atmosphere and solvent-free condition. Its 170.16 h −1 of turnover frequency (TOF) was 2.5 times higher than that of the reported catalyst with the highest TOF value. |
| نوع الوثيقة: | article in journal/newspaper |
| اللغة: | unknown |
| DOI: | 10.3389/fchem.2021.738736 |
| DOI: | 10.3389/fchem.2021.738736/full |
| الاتاحة: | http://dx.doi.org/10.3389/fchem.2021.738736 https://www.frontiersin.org/articles/10.3389/fchem.2021.738736/full |
| Rights: | https://creativecommons.org/licenses/by/4.0/ |
| رقم الانضمام: | edsbas.58BE2871 |
| قاعدة البيانات: | BASE |
| DOI: | 10.3389/fchem.2021.738736 |
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