Photoinduced structural dynamics of multiferroic TbMnO3

التفاصيل البيبلوغرافية
العنوان: Photoinduced structural dynamics of multiferroic TbMnO3
المؤلفون: Abreu, Elsa, id_orcid:0 000-0002-8348-376X, Savoini, Matteo, Boie, Larissa, id_orcid:0 000-0002-1991-3980, Beaud, Paul, Esposito, Vincent, Kubli, Martin, Neugebauer, Martin J., Porer, Michael, Staub, Urs, Burganov, Bulat, Dornes, Christian, Rodriguez-Fernandez, Angel, Huber, Lucas, Lantz, Gabriel, Mardegan, José R.L., Parchenko, Sergii, Rittmann, Jochen, Svetina, Cris, Ingold, Gerhard, Johnson, Steven, id_orcid:0 000-0001-6074-4894
بيانات النشر: ETH Zurich
سنة النشر: 2023
المجموعة: ETH Zürich Research Collection
الوصف: We use time-resolved hard x-ray diffraction to investigate the structural dynamics of the multiferroic insulator TbMnO3 in the low-temperature antiferromagnetic and ferroelectrically ordered phase. The lattice response following photoexcitation at 1.55 eV is detected by measuring the (0 2 4) and (1 3 -5) Bragg reflections. A 0.022% tensile strain, normal to the surface, is seen to arise within 20-40 ps. The magnitude of this transient strain is over an order of magnitude lower than that predicted from laser-induced heating, which we attribute to a bottleneck in the energy transfer between the electronic and lattice subsystems. The timescale for the transient expansion is consistent with that of previously reported demagnetization dynamics. We discuss a possible relationship between structural and demagnetization dynamics in TbMnO3, in which photoinduced atomic motion modulates the exchange interaction, leading to a destruction of the magnetic order in the system.
نوع الوثيقة: dataset
وصف الملف: application/text/plain; application/application/x-matlab-data; application/application/zip
اللغة: English
Relation: http://hdl.handle.net/20.500.11850/587465
DOI: 10.3929/ethz-b-000587465
الاتاحة: https://hdl.handle.net/20.500.11850/587465
https://doi.org/10.3929/ethz-b-000587465
Rights: info:eu-repo/semantics/openAccess ; http://creativecommons.org/licenses/by-sa/4.0/ ; Creative Commons Attribution-ShareAlike 4.0 International
رقم الانضمام: edsbas.4778CE6E
قاعدة البيانات: BASE
الوصف
DOI:10.3929/ethz-b-000587465