Academic Journal

A Fullerene-Platinum Complex for Direct Functional Patterning of Single Metal Atom-Embedded Carbon Nanostructures

التفاصيل البيبلوغرافية
العنوان: A Fullerene-Platinum Complex for Direct Functional Patterning of Single Metal Atom-Embedded Carbon Nanostructures
المؤلفون: Yang, Dongxu, Chen, Xiangyi, He, Dongsheng, Frommhold, Andreas, Shi, Xiaoqing, Boden, Stuart A., Lebedeva, Maria A., Ershova, Olga V., Palmer, Richard E., Li, Ziyou, Shi, Haofei, Gao, Jianzhi, Pan, Minghu, Khlobystov, Andrei N., Chamberlain, Thomas W., Robinson, Alex P. G.
بيانات النشر: American Chemical Society
سنة النشر: 2022
المجموعة: University of Nottingham: Repository@Nottingham
الوصف: The development of patterning materials (“resists”) at the nanoscale involves two distinct trends: one is toward high sensitivity and resolution for miniaturization, the other aims at functionalization of the resists to realize bottom-up construction of distinct nanoarchitectures. Patterning of carbon nanostructures, a seemingly ideal application for organic functional resists, has been highly reliant on complicated pattern transfer processes because of a lack of patternable precursors. Herein, we present a fullerene-metal coordination complex as a fabrication material for direct functional patterning of sub-10 nm metal-containing carbon structures. The attachment of one platinum atom per fullerene molecule not only leads to significant improvement of sensitivity and resolution but also enables stable atomic dispersion of the platinum ions within the carbon matrix, which may gain fundamentally new interest in functional patterning of hierarchical carbon nanostructures.
نوع الوثيقة: article in journal/newspaper
اللغة: English
Relation: https://nottingham-repository.worktribe.com/output/7418310; Journal of Physical Chemistry Letters; Volume 13; Issue 6; Pagination 1578-1586
DOI: 10.1021/acs.jpclett.1c03877
الاتاحة: https://doi.org/10.1021/acs.jpclett.1c03877
https://nottingham-repository.worktribe.com/file/7418310/1/Manuscript-for%20Publication
https://nottingham-repository.worktribe.com/output/7418310
Rights: openAccess
رقم الانضمام: edsbas.1E63D2CD
قاعدة البيانات: BASE
الوصف
DOI:10.1021/acs.jpclett.1c03877