Academic Journal
A Fullerene-Platinum Complex for Direct Functional Patterning of Single Metal Atom-Embedded Carbon Nanostructures
العنوان: | A Fullerene-Platinum Complex for Direct Functional Patterning of Single Metal Atom-Embedded Carbon Nanostructures |
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المؤلفون: | Yang, Dongxu, Chen, Xiangyi, He, Dongsheng, Frommhold, Andreas, Shi, Xiaoqing, Boden, Stuart A., Lebedeva, Maria A., Ershova, Olga V., Palmer, Richard E., Li, Ziyou, Shi, Haofei, Gao, Jianzhi, Pan, Minghu, Khlobystov, Andrei N., Chamberlain, Thomas W., Robinson, Alex P. G. |
بيانات النشر: | American Chemical Society |
سنة النشر: | 2022 |
المجموعة: | University of Nottingham: Repository@Nottingham |
الوصف: | The development of patterning materials (“resists”) at the nanoscale involves two distinct trends: one is toward high sensitivity and resolution for miniaturization, the other aims at functionalization of the resists to realize bottom-up construction of distinct nanoarchitectures. Patterning of carbon nanostructures, a seemingly ideal application for organic functional resists, has been highly reliant on complicated pattern transfer processes because of a lack of patternable precursors. Herein, we present a fullerene-metal coordination complex as a fabrication material for direct functional patterning of sub-10 nm metal-containing carbon structures. The attachment of one platinum atom per fullerene molecule not only leads to significant improvement of sensitivity and resolution but also enables stable atomic dispersion of the platinum ions within the carbon matrix, which may gain fundamentally new interest in functional patterning of hierarchical carbon nanostructures. |
نوع الوثيقة: | article in journal/newspaper |
اللغة: | English |
Relation: | https://nottingham-repository.worktribe.com/output/7418310; Journal of Physical Chemistry Letters; Volume 13; Issue 6; Pagination 1578-1586 |
DOI: | 10.1021/acs.jpclett.1c03877 |
الاتاحة: | https://doi.org/10.1021/acs.jpclett.1c03877 https://nottingham-repository.worktribe.com/file/7418310/1/Manuscript-for%20Publication https://nottingham-repository.worktribe.com/output/7418310 |
Rights: | openAccess |
رقم الانضمام: | edsbas.1E63D2CD |
قاعدة البيانات: | BASE |
DOI: | 10.1021/acs.jpclett.1c03877 |
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