Report
Optically Induced Avoided Crossing in Graphene
العنوان: | Optically Induced Avoided Crossing in Graphene |
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المؤلفون: | Buchenau, Sören, Grimm-Lebsanft, Benjamin, Biebl, Florian, Glier, Tomke, Westphal, Lea, Reichstetter, Janika, Manske, Dirk, Fechner, Michael, Cavalleri, Andrea, Herres-Pawlis, Sonja, Rübhausen, Michael |
سنة النشر: | 2023 |
المجموعة: | Condensed Matter Physics (Other) |
مصطلحات موضوعية: | Condensed Matter - Materials Science, Physics - Optics |
الوصف: | Degenerate states in condensed matter are frequently the cause of unwanted fluctuations, which prevent the formation of ordered phases and reduce their functionalities. Removing these degeneracies has been a common theme in materials design, pursued for example by strain engineering at interfaces. Here, we explore a non-equilibrium approach to lift degeneracies in solids. We show that coherent driving of the crystal lattice in bi- and multilayer graphene, boosts the coupling between two doubly-degenerate modes of E1u and E2g symmetry, which are virtually uncoupled at equilibrium. New vibronic states result from anharmonic driving of the E1u mode to large amplitdues, boosting its coupling to the E2g mode. The vibrational structure of the driven state is probed with time-resolved Raman scattering, which reveals laser-field dependent mode splitting and enhanced lifetimes. We expect this phenomenon to be generally observable in many materials systems, affecting the non-equilibrium emergent phases in matter. Comment: 13 pages, 4 figures |
نوع الوثيقة: | Working Paper |
URL الوصول: | http://arxiv.org/abs/2307.11562 |
رقم الانضمام: | edsarx.2307.11562 |
قاعدة البيانات: | arXiv |
الوصف غير متاح. |