Two and three photon excited luminescence of single gold nanoparticles: Switching between plasmon- and electron-hole-pair emission by ultrashort laser pulses

التفاصيل البيبلوغرافية
العنوان: Two and three photon excited luminescence of single gold nanoparticles: Switching between plasmon- and electron-hole-pair emission by ultrashort laser pulses
المؤلفون: Wackenhut, Frank, Wang, Xiao, Failla, Antonio Virgilio, Meixner, Alfred J.
سنة النشر: 2018
المجموعة: Physics (Other)
مصطلحات موضوعية: Physics - Optics
الوصف: In this work we use femtosecond laser pulses of 800 nm wavelength to excite and characterize the multiphoton luminescence emission of single gold nanoparticles. For excitation with 100 fs laser pulses we observe a two and three photon emission dominated by radiative electron hole pair recombination, while the emission is caused by radiative plasmon decay for excitation with 500 fs pulses. For single gold nanorods with different aspect ratios, we study the interplay between the particle plasmon and electron hole pairs, which enables us to develop a quantitative model to fully describe the two and three photon luminescence emission of single gold nanoparticles.
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/1812.01409
رقم الانضمام: edsarx.1812.01409
قاعدة البيانات: arXiv