Ferromagnetism induced by orbital order in the charge-transfer insulator Cs2AgF4: an electronic structure study

التفاصيل البيبلوغرافية
العنوان: Ferromagnetism induced by orbital order in the charge-transfer insulator Cs2AgF4: an electronic structure study
المؤلفون: Deepa, Kasinathan, Klaus, Koepernik, Ulrike, Nitzsche, Helge, Rosner
المصدر: Physical review letters. 99(24)
سنة النشر: 2007
الوصف: Cs2AgF4 was proposed to be an orbitally ordered ferromagnet based on recent neutron scattering data. Here, we report a detailed electronic structure study within the local spin density approximation also including strong Coulomb repulsion U. We investigate the influence of an orthorhombic distortion of the Ag environment and the importance of the on-site Coulomb repulsion. We find good quantitative agreement with both the experimentally observed exchange coupling and structural changes. Thus, our results strongly support that Cs2AgF4 is a strongly correlated charge-transfer insulator where the ferromagnetism is driven by orbital order.
تدمد: 0031-9007
URL الوصول: https://explore.openaire.eu/search/publication?articleId=pmid________::597697e23f34ac71955bc0c1a92efe13
https://pubmed.ncbi.nlm.nih.gov/18233485
رقم الانضمام: edsair.pmid..........597697e23f34ac71955bc0c1a92efe13
قاعدة البيانات: OpenAIRE