Near-ifrared-II photodetectors based on silver selenide quantum dots on mesoporous TiO₂ scaffolds

التفاصيل البيبلوغرافية
العنوان: Near-ifrared-II photodetectors based on silver selenide quantum dots on mesoporous TiO₂ scaffolds
المؤلفون: Graddage, Neil, Ouyang, Jianying, Lu, Jianping, Chu, Ta-Ya, Zhang, Yanguang, Li, Zhao, Wu, Xiaohua, Malenfant, Patrick R. L., Tao, Ye
بيانات النشر: American Chemical Society, 2021.
سنة النشر: 2021
مصطلحات موضوعية: photodiode structures, photodetectors, Ag2Se colloidal quantum dots, mesoporous TiO2 scaffold, solution processing, second near-infrared window
الوصف: Biosensing applications are driving an increase in demand for low-cost photodetectors with sensitivity between 1000 and 1400 nm. Recently, the sensitivity of Ag₂Se colloidal quantum dot based devices in this wavelength range has been observed. In this work we make the first demonstration of an Ag₂Se photodiode device with sensitivity in this entire range. By employing secondary phosphine to elevate the precursor reactivity, we achieved accurate size control of the Ag₂Se nanocrystals with a distinct excitonic absorption peak. These nanocrystals were deposited from solution into a mesoporous TiO₂ scaffold, similar to that used in dye-sensitized solar cells, to increase the light absorption and charge separation and reduce the exciton diffusion length. By incorporation of a suitable hole-transporting layer between the active layer and Ag anode, the resulting devices showed a responsivity of 4.17 mA/W at a wavelength of 1200 nm. These results demonstrate that Ag₂Se colloidal quantum dots offer a low-toxicity route for low-cost fabrication of near-infrared photodetectors.
وصف الملف: application/pdf
اللغة: English
URL الوصول: https://explore.openaire.eu/search/publication?articleId=od______1674::5570e59e743ef91f0bcb022fecc6c45c
https://nrc-publications.canada.ca/eng/view/object/?id=e288c20d-6cd6-4e8f-a241-64b6dfe7651b
Rights: OPEN
رقم الانضمام: edsair.od......1674..5570e59e743ef91f0bcb022fecc6c45c
قاعدة البيانات: OpenAIRE