Chemical stability of 2-arachidonylglycerol under biological conditions

التفاصيل البيبلوغرافية
العنوان: Chemical stability of 2-arachidonylglycerol under biological conditions
المؤلفون: Kebreab Ghebreselasie, Lawrence J. Marnett, Carol A. Rouzer
المصدر: Chemistry and Physics of Lipids. 119:69-82
بيانات النشر: Elsevier BV, 2002.
سنة النشر: 2002
مصطلحات موضوعية: Tris, Receptors, Drug, Arachidonic Acids, Buffers, Ligands, Biochemistry, High-performance liquid chromatography, Glycerides, chemistry.chemical_compound, Drug Stability, Molecule, Receptors, Cannabinoid, Molecular Biology, Incubation, Chromatography, High Pressure Liquid, Detection limit, Chromatography, Ligand, Organic Chemistry, Cell Biology, Culture Media, chemistry, Ionic strength, Chemical stability, Oxidation-Reduction, Endocannabinoids
الوصف: Recent evidence indicates that 2-arachidonylglycerol (2-AG) is a potent and specific ligand for the central and peripheral cannabinoid receptors. Therefore, the chemical stability of this molecule under biological conditions is of interest. A method for the isolation and detection of 2-AG using HPLC with evaporative light scattering detection is described. The method provides an extraction recovery from aqueous media of 78%, and a limit of detection of 60 ng on column. Incubation of 2-AG in culture medium or biological buffers indicated that it is stable to oxidation and ester hydrolysis for up to 6 h at 37 degrees C. However, gradual disappearance of the compound was noted due to adherence to glass and plastic surfaces. During incubation in RPMI culture medium, 2-AG rearranged to 1(3)-arachidonylglycerol (1(3)-AG) in a first order process with a half-life of 10 min in the absence of serum and 2.3 min in the presence of 10% fetal calf serum. Further studies indicated that the acyl migration reaction is base catalyzed (k(cat)=78,000/min M), and that the reaction is affected slightly by changes in buffer (Tris) concentration and not at all by changes in ionic strength. The results indicate that 2-AG is readily converted to 1(3)-AG under conditions commonly used to study receptor-ligand interactions, findings that have significant implications for the interpretation of relative ligand potency between the two isomers.
تدمد: 0009-3084
DOI: 10.1016/s0009-3084(02)00068-3
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::aa6e9c98b13efa06a1b02d1f5726b009
https://doi.org/10.1016/s0009-3084(02)00068-3
Rights: CLOSED
رقم الانضمام: edsair.doi.dedup.....aa6e9c98b13efa06a1b02d1f5726b009
قاعدة البيانات: OpenAIRE
الوصف
تدمد:00093084
DOI:10.1016/s0009-3084(02)00068-3