Identification of 6-benzyloxysalicylates as a novel class of inhibitors of 15-lipoxygenase-1

التفاصيل البيبلوغرافية
العنوان: Identification of 6-benzyloxysalicylates as a novel class of inhibitors of 15-lipoxygenase-1
المؤلفون: Johan te Biesebeek, Frank J. Dekker, Stephanie Thee, Nikolaos Eleftheriadis, Bert-Jan Baas, Petra E van der Wouden
المساهمون: Biopharmaceuticals, Discovery, Design and Delivery (BDDD), Medicinal Chemistry and Bioanalysis (MCB)
المصدر: European Journal of Medicinal Chemistry, 94, 265-275. ELSEVIER MASSON, CORPORATION OFFICE
سنة النشر: 2015
مصطلحات موضوعية: Models, Molecular, Chronic bronchitis, Kinetic analysis, Pharmacology, Lipoxygenase, Structure-Activity Relationship, Non-competitive inhibition, Drug Discovery, Arachidonate 15-Lipoxygenase, Humans, Enzyme kinetics, Lipoxygenase Inhibitors, chemistry.chemical_classification, biology, Dose-Response Relationship, Drug, Molecular Structure, Chemistry, Drug discovery, Organic Chemistry, food and beverages, General Medicine, Salicylates, Kinetics, Enzyme, Biochemistry, biology.protein, Polyunsaturated fatty acid
الوصف: Lipoxygenases metabolize polyunsaturated fatty acids into signalling molecules such as leukotrienes and lipoxins. 15-lipoxygenase-1 (15-LOX-1) is an important mammalian lipoxygenase and plays a crucial regulatory role in several respiratory diseases such as asthma, COPD and chronic bronchitis. Novel potent and selective inhibitors of 15-LOX-1 are required to explore the role of this enzyme in drug discovery. In this study we describe structure activity relationships for 6-benzyloxysalicylates as inhibitors of human 15-LOX-1. Kinetic analysis suggests competitive inhibition and the binding model of these compounds can be rationalized using molecular modelling studies. The most potent derivative 37a shows a Ki value of 1.7 μM. These structure activity relationships provide a basis to design improved inhibitors and to explore 15-LOX-1 as a drug target.
وصف الملف: application/pdf
اللغة: English
تدمد: 0223-5234
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::6c5795680e040feb218329921d0320b3
https://hdl.handle.net/11370/b2c5a254-1979-4eb4-829d-9b35baa1aa33
Rights: OPEN
رقم الانضمام: edsair.doi.dedup.....6c5795680e040feb218329921d0320b3
قاعدة البيانات: OpenAIRE