Experimental values for 241Am and 239+240Pu Kd's in French agricultural soils

التفاصيل البيبلوغرافية
العنوان: Experimental values for 241Am and 239+240Pu Kd's in French agricultural soils
المؤلفون: Sylvie Roussel-Debet
المصدر: Journal of Environmental Radioactivity. 79:171-185
بيانات النشر: Elsevier BV, 2005.
سنة النشر: 2005
مصطلحات موضوعية: Health, Toxicology and Mutagenesis, chemistry.chemical_element, Americium, Soil science, Soil, Plutonium-240, Soil pH, Soil Pollutants, Radioactive, Environmental Chemistry, Waste Management and Disposal, Agriculture, Sorption, General Medicine, Hydrogen-Ion Concentration, Models, Theoretical, Pollution, Soil contamination, Plutonium, Partition coefficient, Kinetics, chemistry, Soil water, Adsorption, France, Plutonium-239, Power Plants, Nuclear chemistry
الوصف: Experiments resulted in determination of K d values for 241 Am and 239+240 Pu in 6 soils whose characteristics are representative of agricultural soils found around French nuclear power plant sites. These experiments were conducted in stirred batch reactors and the sorption isotherms were plotted. For americium, the experimental K d values varied from 60 to 4000 L kg −1 (d.w.) and correlated well with soil pH, K d increased with increasing pH. As regards plutonium, the experimental K d values varied between 300 and 9600 L kg −1 and decreased with increasing total sand content. The estimation of the total residence time determined by using a particular and experimentally refined value for K d —with a model similar to those currently used for impact assessments—illustrates the importance of establishing values that are better suited to specific soils than generic values. Lastly, depending on the type of evaluation envisioned, it might be important to look for a specific value of K d —and even modelling—more suited to the specificity of the scenario studied, by performing more complex, or even in situ, experiments.
تدمد: 0265-931X
DOI: 10.1016/j.jenvrad.2004.06.004
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::4d2c0e729768abd50b3663bafcdeca33
https://doi.org/10.1016/j.jenvrad.2004.06.004
Rights: CLOSED
رقم الانضمام: edsair.doi.dedup.....4d2c0e729768abd50b3663bafcdeca33
قاعدة البيانات: OpenAIRE
الوصف
تدمد:0265931X
DOI:10.1016/j.jenvrad.2004.06.004