An approach to incorporate multiple forms of iodine in radiological consequence analysis

التفاصيل البيبلوغرافية
العنوان: An approach to incorporate multiple forms of iodine in radiological consequence analysis
المؤلفون: Sung-yeop Kim, Nathan E. Bixler, Seok-Won Hwang, Kwang-Il Ahn
المصدر: Journal of environmental radioactivity. 213
سنة النشر: 2019
مصطلحات موضوعية: Chemical substance, 010504 meteorology & atmospheric sciences, Multiple forms, Health, Toxicology and Mutagenesis, Radiochemistry, chemistry.chemical_element, General Medicine, 010501 environmental sciences, Iodides, Iodine, 01 natural sciences, Pollution, Aerosol, Iodine Radioisotopes, Deposition (aerosol physics), chemistry, ORGANIC IODIDE, Air Pollutants, Radioactive, Radiation Monitoring, Air concentration, Environmental Chemistry, Consequence analysis, Waste Management and Disposal, 0105 earth and related environmental sciences
الوصف: Interest is increasing in the radiological consequences of a release of aerosol and gaseous iodine, especially after the Fukushima accident and also because of new interpretations of the results of recent severe accident experiments. This work provides a brief review of the history of iodine chemistry in containment and suggests an approach to include gaseous iodine, namely in the forms of elemental iodine and organic iodide, in consequence analyses using the MACCS code. As dry deposition is an important characteristic to distinguish each chemical form of iodine when performing a consequence analysis, the mechanisms and mathematical formulas expressing dry deposition are also investigated. The proposed approach is demonstrated by performing consequence analyses with a unit release of 131I, with the resulting trends of concentration and dose for the different chemical forms of iodine presented and discussed. For the same amount of iodine release, there is a higher surface deposition of elemental iodine (I2) because it has a higher dry deposition velocity, while the air concentration of a representative organic iodide (CH3I) is higher due to its lower dry deposition velocity, which means a lower depletion of the air concentration. Despite elemental iodine having a lower air concentration, its higher dose coefficients for the inhalation pathway compensates for this when calculating doses. Further, inhaled doses increase when considering resuspension inhalation for extended durations of exposure. The approach proposed in this study is expected to be used flexibly to perform consequence analyses incorporating both aerosol and gaseous forms of iodine.
تدمد: 1879-1700
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::320d0ccae92c15785424698b17aa8960
https://pubmed.ncbi.nlm.nih.gov/31983448
Rights: CLOSED
رقم الانضمام: edsair.doi.dedup.....320d0ccae92c15785424698b17aa8960
قاعدة البيانات: OpenAIRE