Insulating phase in Sr2IrO4: An investigation using critical analysis and magnetocaloric effect

التفاصيل البيبلوغرافية
العنوان: Insulating phase in Sr2IrO4: An investigation using critical analysis and magnetocaloric effect
المؤلفون: Imtiaz Noor Bhatti, Ashim Pramanik
المصدر: Journal of Magnetism and Magnetic Materials. 422:141-148
بيانات النشر: Elsevier BV, 2017.
سنة النشر: 2017
مصطلحات موضوعية: Materials science, Strongly Correlated Electrons (cond-mat.str-el), Condensed matter physics, Demagnetizing field, FOS: Physical sciences, 02 engineering and technology, Spin–orbit interaction, Renormalization group, 021001 nanoscience & nanotechnology, Condensed Matter Physics, 01 natural sciences, Electronic, Optical and Magnetic Materials, Condensed Matter - Strongly Correlated Electrons, Spin wave, Electrical resistivity and conductivity, 0103 physical sciences, Magnetic refrigeration, Condensed Matter::Strongly Correlated Electrons, 010306 general physics, 0210 nano-technology, Critical exponent, Scaling
الوصف: The nature of insulating phase in 5$d$ based Sr$_2$IrO$_4$ is quite debated as the theoretical as well as experimental investigations have put forward evidences in favor of both magnetically driven Slater-type and interaction driven Mott-type insulator. To understand this insulating behavior, we have investigated the nature of magnetic state in Sr$_2$IrO$_4$ through studying critical exponents, low temperature thermal demagnetization and magnetocaloric effect. The estimated critical exponents do not exactly match with any universality class, however, the values obey the scaling behavior. The exponent values suggest that spin interaction in present material is close to mean-field model. The analysis of low temperature thermal demagnetization data, however, shows dual presence of localized- and itinerant-type of magnetic interaction. Moreover, field dependent change in magnetic entropy indicates magnetic interaction is close to mean-field type. While this material shows an insulating behavior across the magnetic transition, yet a distinct change in slope in resistivity is observed around $T_c$. We infer that though the insulating phase in Sr$_2$IrO$_4$ more close to be Slater-type but the simultaneous presence of both Slater- and Mott-type is the likely scenario for this material.
تدمد: 0304-8853
DOI: 10.1016/j.jmmm.2016.08.065
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::2dd00a5f0b2096015dcc748dfeb814ee
https://doi.org/10.1016/j.jmmm.2016.08.065
Rights: OPEN
رقم الانضمام: edsair.doi.dedup.....2dd00a5f0b2096015dcc748dfeb814ee
قاعدة البيانات: OpenAIRE
الوصف
تدمد:03048853
DOI:10.1016/j.jmmm.2016.08.065