Concerning the mechanism for transfer of D-glucuronate from myo-inositol oxygenase to D-glucuronate reductase

التفاصيل البيبلوغرافية
العنوان: Concerning the mechanism for transfer of D-glucuronate from myo-inositol oxygenase to D-glucuronate reductase
المؤلفون: Gordon A. Hamilton, Nariman I. Naber
المصدر: Biochimica et biophysica acta. 911(3)
سنة النشر: 1987
مصطلحات موضوعية: chemistry.chemical_classification, Oxygenase, Stereochemistry, Glucuronate, Inositol Oxygenase, Biophysics, Glucuronates, Glucuronate reductase, Reductase, NADPH oxidation, Biochemistry, Inositol oxygenase, chemistry.chemical_compound, Kinetics, Enzyme, Oxygen Consumption, chemistry, Glucuronic Acid, Structural Biology, Oxygenases, Hemiacetal, Carbohydrate Dehydrogenases, Molecular Biology, NADP
الوصف: The D-glucuronate product of myo-inositol oxygenase (EC 1.13.99.1) is efficiently reduced by NADPH in the presence of either purified D-glucuronate reductase (EC 1.1.1.19), or reductase that is part of a protein aggregate that also contains the oxygenase. This occurs despite the fact that the maximum concentration of D-glucuronate that could be formed by the oxygenase under the conditions used for the coupled enzyme experiments is 7 microM, and 10 microM externally supplied D-glucuronate (Km = 7.6 mM) does not support any detectable NADPH oxidation under the reaction conditions. The most likely explanation for the results is that the uncyclized aldehyde form of D-glucuronate is the product of the oxygenase reaction, and that it diffuses into solution and is captured by the reductase before it cyclizes to the more stable but less reactive hemiacetal form.
تدمد: 0006-3002
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::2d56871772985581531747c712a28207
https://pubmed.ncbi.nlm.nih.gov/3814609
Rights: CLOSED
رقم الانضمام: edsair.doi.dedup.....2d56871772985581531747c712a28207
قاعدة البيانات: OpenAIRE