Strong-field-gated buildup of a Rydberg series

التفاصيل البيبلوغرافية
العنوان: Strong-field-gated buildup of a Rydberg series
المؤلفون: Thomas Pfeifer, Gergana Dimitrova Borisova, Paul Birk, Maximilian Hartmann, Veit Stooß, Alexander Blättermann, Christian D. Ott
المصدر: Physical Review Research
سنة النشر: 2020
مصطلحات موضوعية: Physics, Series (mathematics), chemistry.chemical_element, Strong field, 01 natural sciences, Spectral line, 010305 fluids & plasmas, symbols.namesake, chemistry, Excited state, 0103 physical sciences, Rydberg formula, symbols, Physics::Atomic and Molecular Clusters, Physics::Atomic Physics, Physics::Chemical Physics, Atomic physics, 010306 general physics, Absorption (electromagnetic radiation), Ultrashort pulse, Helium
الوصف: The femtosecond-timescale formation of a Fano resonance in doubly excited helium has been recently observed, enabling a time-domain view into two-electron correlation dynamics. Measuring the absorption spectral line shape, the buildup of the resonance is revealed by imposing a temporal gate on the dipole response using strong-field ionization. Here, we apply this approach to the Rydberg series of the doubly excited states in helium. This reveals the characteristic times of emergence of isolated two-electron resonances from the continuous single-ionization background absorption, as well as their time-dependent line-shape asymmetry and the time it takes to separate individual spectral absorption lines within the series. Furthermore, we time resolve the dynamics of the excited wave packet by reconstructing its dipole response in the time domain and thereby characterize the ionization gate to close as fast as only 1.2 fs. These results represent an approach to resolve on the femtosecond and attosecond timescale the strong-field-ionization dynamics of excited coherent wave packets.
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::2480f05518b56a235b3684347c7c7e16
https://hdl.handle.net/21.11116/0000-0007-147D-7
Rights: OPEN
رقم الانضمام: edsair.doi.dedup.....2480f05518b56a235b3684347c7c7e16
قاعدة البيانات: OpenAIRE