Sampling, on-line and off-line measurement of organic silicon compounds at an industrial biogas-fed 175-kWe SOFC plant

التفاصيل البيبلوغرافية
العنوان: Sampling, on-line and off-line measurement of organic silicon compounds at an industrial biogas-fed 175-kWe SOFC plant
المؤلفون: Dita Heikens, Adelaide Calbry-Muzyka, Serge M.A. Biollaz, Jianrong Li, Mohamed Tarik, Christian Ludwig, Debora Foppiano, Iris de Krom, Marta Gandiglio
مصطلحات موضوعية: Spectrum analyzer, Sorbent, Silicon, Siloxanes, 020209 energy, chemistry.chemical_element, 02 engineering and technology, Biogas cleaning, Adsorption, Online analysis, Biogas, Nondispersive infrared sensor, 0202 electrical engineering, electronic engineering, information engineering, 0601 history and archaeology, Process engineering, NDIR, 060102 archaeology, Renewable Energy, Sustainability and the Environment, business.industry, Sampling (statistics), 06 humanities and the arts, GC-ICP-MS, GC-FID, chemistry, Environmental science, Solid oxide fuel cell, business
الوصف: The use of biogas in the energy sector requires efficient removal of harmful trace levels of impurities. Reliable and robust online analytical equipment to measure these impurities is necessary and must be validated using offline techniques. In this work, total silicon and siloxanes were measured at an industrial solid oxide fuel cell fed by biogas. SOFC anodes are sensitive to silicon-based contaminants even at parts-per-billion levels. Online measurements of total silicon were carried out using a nondispersive infrared sensor (NDIR). Different sampling methods, including chemical adsorption, liquid quenching, and solid-phase adsorption were used at six biogas sampling points. Organic silicon compounds in the samples were determined by offline methods including GC-FID and GC-ICP-MS. The online analyzer's performance was satisfactory in both untreated biogas, where it agreed within the error margin of the most reliable offline technique used, and in clean biogas, where
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::14f49731d27cfafd006adfe157d3d837
https://infoscience.epfl.ch/record/285997
Rights: OPEN
رقم الانضمام: edsair.doi.dedup.....14f49731d27cfafd006adfe157d3d837
قاعدة البيانات: OpenAIRE