Impedance spectroscopy and conduction mechanism of a BiFe$_{0.95}$Mn$_{0.05}$O$_3$ thin film

التفاصيل البيبلوغرافية
العنوان: Impedance spectroscopy and conduction mechanism of a BiFe$_{0.95}$Mn$_{0.05}$O$_3$ thin film
المؤلفون: S. Yousfi, Houssny Bouyanfif, M. El Marssi
سنة النشر: 2021
مصطلحات موضوعية: Materials science, FOS: Physical sciences, 02 engineering and technology, Dielectric, 7. Clean energy, 01 natural sciences, Condensed Matter::Materials Science, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), 0103 physical sciences, Materials Chemistry, Thin film, Electrical impedance, 010302 applied physics, Condensed Matter - Materials Science, Condensed matter physics, Condensed Matter - Mesoscale and Nanoscale Physics, Direct current, Metals and Alloys, Materials Science (cond-mat.mtrl-sci), Surfaces and Interfaces, 021001 nanoscience & nanotechnology, Thermal conduction, Space charge, Surfaces, Coatings and Films, Electronic, Optical and Magnetic Materials, Dielectric spectroscopy, Relaxation (physics), 0210 nano-technology
الوصف: Dielectric response and conduction mechanism were investigated for a multiferroic BiFe$_{0.95}$Mn$_{0.05}$O$_3$ epitaxial thin film. A contribution from a thermally activated interface (0.37 eV) and the bulk of the film on the dielectric response were observed through the comparison between experimental results and equivalent circuit model. The low frequency interface relaxation signatures strongly suggest a Maxwell-Wagner space charge origin. The alternative current conductivity deduced from the model follows a power law frequency dependence suggesting a polaronic hopping mechanism while the low frequency limit is in perfect agreement with the direct current conduction mechanism. The current-voltage characteristics were indeed correlated with Schottky-Simmons interface limited transport with activation energy of 0.36 eV, close to the one extracted from the impedance analysis. Such analysis of the electrostatic landscape and dielectric behaviour may help to further understanding the anomalous photo-induced properties in the BiFeO$_3$ system.
اللغة: English
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::10eb2c2179ca8727a889e072b97059a5
http://arxiv.org/abs/2103.04115
Rights: OPEN
رقم الانضمام: edsair.doi.dedup.....10eb2c2179ca8727a889e072b97059a5
قاعدة البيانات: OpenAIRE