Evaluation of a C18 hybrid stationary phase using high-temperature chromatography

التفاصيل البيبلوغرافية
العنوان: Evaluation of a C18 hybrid stationary phase using high-temperature chromatography
المؤلفون: Karen C. Thompson, John E. O'Gara, Thomas H. Walter, Y. Liu, R.M. Wenslow, Kevin D. Wyndham, Nelu Grinberg, D. Morrison, Uwe D. Neue
المصدر: Analytica Chimica Acta. 554:144-151
بيانات النشر: Elsevier BV, 2005.
سنة النشر: 2005
مصطلحات موضوعية: Van Deemter equation, chemistry.chemical_classification, Analyte, Phase transition, Chromatography, Analytical chemistry, Biochemistry, Toluene, Analytical Chemistry, chemistry.chemical_compound, Differential scanning calorimetry, chemistry, Phase (matter), Environmental Chemistry, Benzene, Spectroscopy, Alkyl
الوصف: Alkyl benzenes and aromatic alcohols were used as model analytes in a chromatographic separation on a new type of hybrid C18 stationary phase. The stationary phase was characterized from the point of view of its interaction with the mentioned analytes. The thermodynamic parameters such as Δ H ° and Δ S ° showed that there are very few differences in the interactions of the alkyl benzenes and aromatic alcohols with the stationary phase in the temperature interval from 150 to 200 °C. A temperature study in the range from 30 to 200 °C using toluene as an analyte revealed that the van’t Hoff plot is non-linear. Differential scanning calorimetry studies on this stationary phase indicated a phase transition at ∼90 °C. Studies on the influence of organic modifier concentrations indicated that the retention of the analytes at 150 °C varied linearly with the volume fraction of acetonitrile in the mobile phase. At 150 °C the van Deemter plot showed that a minimum was reached for the reduced plate height at ∼1.6 mL/min which was constant up to 5 mL/min. A 1-month stability study of the column using pure water as a mobile phase, at 200 °C indicated that analyte retention factor changed by 10% during this period of time.
تدمد: 0003-2670
DOI: 10.1016/j.aca.2005.08.026
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::fcaa5b6f02f95bbada85fb50591dc3f9
https://doi.org/10.1016/j.aca.2005.08.026
Rights: CLOSED
رقم الانضمام: edsair.doi...........fcaa5b6f02f95bbada85fb50591dc3f9
قاعدة البيانات: OpenAIRE
الوصف
تدمد:00032670
DOI:10.1016/j.aca.2005.08.026