F2, H2O, and O2 etching rates of diamond and the effects of F2, HF and H2O on the molecular O2 etching of (110) diamond

التفاصيل البيبلوغرافية
العنوان: F2, H2O, and O2 etching rates of diamond and the effects of F2, HF and H2O on the molecular O2 etching of (110) diamond
المؤلفون: Robert H. Hauge, C. Pan, J. L. Margrave, C. J. Chu
المصدر: Diamond and Related Materials. 4:1317-1324
بيانات النشر: Elsevier BV, 1995.
سنة النشر: 1995
مصطلحات موضوعية: Vapor pressure, Mechanical Engineering, Inorganic chemistry, Diamond, chemistry.chemical_element, General Chemistry, engineering.material, Hydrogen fluoride, Oxygen, Isotropic etching, Electronic, Optical and Magnetic Materials, chemistry.chemical_compound, Hydrofluoric acid, chemistry, Etching (microfabrication), Materials Chemistry, engineering, Fluorine, Electrical and Electronic Engineering
الوصف: Oxidation kinetics of natural (110) diamond by oxygen and water were investigated using in situ Fizeau interferometry. Apparent activation energies of 53 and 26 kcal mol −1 were obtained for the etching of (110) type Ia diamond by O 2 and H 2 O respectively. The etch rate was found to follow second-order kinetics with respect to O 2 pressure in the pressure range 0.04–10 Torr. For water over the vapour pressure range 0.1–2 Torr, the reaction has a reaction order near unity. The diamond (110) surface was impervious to etching by molecular fluorine at all temperatures up to 1300 °C. Fluorine, hydrogen fluoride and water were found to inhibit the molecular oxygen etching of diamond. Below 900 °C, oxidation is inhibited by the addition of F 2 and HF presumably by blocking reactive sites on the diamond surface through formation of CF bonds. Above 900 °C, the fluorine is thought to desorb from the diamond (110) surface, rendering the surface susceptible to further oxidation. Addition of water below 800 °C was found to retard etching by molecular oxygen. This is attributed to the formation of COH bonds, analogous to CF.
تدمد: 0925-9635
DOI: 10.1016/0925-9635(95)00311-8
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::b1558d88b57aebe52ce15955cadc1ed7
https://doi.org/10.1016/0925-9635(95)00311-8
Rights: CLOSED
رقم الانضمام: edsair.doi...........b1558d88b57aebe52ce15955cadc1ed7
قاعدة البيانات: OpenAIRE
الوصف
تدمد:09259635
DOI:10.1016/0925-9635(95)00311-8