Thermodynamics of Lithium-Ion Batteries

التفاصيل البيبلوغرافية
العنوان: Thermodynamics of Lithium-Ion Batteries
المؤلفون: Rachid Yazami, Kenza Maher
بيانات النشر: Elsevier, 2014.
سنة النشر: 2014
مصطلحات موضوعية: Phase transition, Overcharge, Materials science, law, Enthalpy, Thermodynamics, Capacity loss, Cobalt oxide, Cathode, Anode, law.invention, Ion
الوصف: Li-ion batteries (LiB) of coin-cell form factor (2032) were subjected to three different accelerate aging modes; i. overcharge ageing up to 4.9 V end of charge cut-off voltages (COV), ii. thermal aging at 60 °C and 70 °C for a period of up to 8 weeks after being charged to 4.2 V at ambient temperatures , and iii. long cycling at a C/2 rate at ambient temperature for up to 1000 cycles. We found the entropy (ΔS) and enthalpy (ΔH) profiles varied with aging conditions much more readily than open-circuit potential (OCP) profiles. We also found that aged batteries keep a thermodynamic fingerprint of the process by which they aged. This memory effect can be revealed by measuring the entropy and enthalpy of aged cells at two particular OCP of 3.87 V and OCP = 3.94 V, which are specific to LiB based on graphite anode and lithiated cobalt oxide (LCO) cathode material. In fact 3.87 V and 3.94 V are potentials of phase transition in the anode and cathode materials, respectively. Another aspect of the thermodynamics memory effect is a characteristic change of entropy and enthalpy profiles of cells having incurred the same capacity loss under different aging modes as compared to almost identical OCP and discharge profiles.
DOI: 10.1016/b978-0-444-59513-3.00025-x
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::78ebf0695f02032d35aff43101781abd
https://doi.org/10.1016/b978-0-444-59513-3.00025-x
رقم الانضمام: edsair.doi...........78ebf0695f02032d35aff43101781abd
قاعدة البيانات: OpenAIRE
الوصف
DOI:10.1016/b978-0-444-59513-3.00025-x