A novel thermostable and halotolerant xylanase from Colletotrichum graminicola

التفاصيل البيبلوغرافية
العنوان: A novel thermostable and halotolerant xylanase from Colletotrichum graminicola
المؤلفون: Luiz Alberto Beraldo de Moraes, Luana Parras Meleiro, José César Rosa, João Atílio Jorge, Sibeli Carli, Douglas Chodi Masui, Rosa dos Prazeres Melo Furriel
المصدر: Journal of Molecular Catalysis B: Enzymatic. 133:S508-S517
بيانات النشر: Elsevier BV, 2016.
سنة النشر: 2016
مصطلحات موضوعية: 0106 biological sciences, 0301 basic medicine, Chromatography, Process Chemistry and Technology, Size-exclusion chromatography, Bioengineering, 01 natural sciences, Biochemistry, Catalysis, 03 medical and health sciences, chemistry.chemical_compound, Hydrolysis, 030104 developmental biology, chemistry, 010608 biotechnology, Halotolerance, Xylobiose, Xylanase, Sodium dodecyl sulfate, Polyacrylamide gel electrophoresis, Sodium acetate
الوصف: A novel endoxylanase from Colletotrichum graminicola (Excg1) was purified. Similar apparent molecular masses were estimated by gel filtration (17.3 ± 1.9 kDa) and sodium dodecyl sulfate polyacrylamide gel electrophoresis (20.0 ± 2.4 kDa), suggesting that Excg1 is monomeric. The enzyme showed good halotolerance, retaining about 85% and 50% of the control activity in the presence of 0.5 mol L−1 and 3.0 mol L−1 NaCl, respectively. The optimum temperature of Excg1 (65 °C) was not affected by NaCl, but the optimum pH rose from 5.5 in the absence and presence of 0.5 mol L−1 NaCl to 6.0, in 2.5 mol L−1 NaCl. Excg1 was highly thermostable at 50 °C, with half-lives around 48 h in either water or 0.5 mol L−1 NaCl and a residual activity of 75% at 2.5 mol L−1 NaCl. Excg1 was fully stable at pH 3.0–10.0 in the absence of salt, and from pH 4.0–10.0 in the presence of 0.5 mol L−1 and 2.5 mol L−1 NaCl. The enzyme hydrolyzed beechwood xylan with maximal velocity and apparent affinity constant of 481.3 ± 34.0 U mg−1 and 3.7 ± 0.3 mg mL−1, respectively. Similar kinetic parameters were obtained in the presence of 0.5 mol L−1 NaCl, but a maximum velocity about 34% lower was determined in 2.5 mol L−1 NaCl. Excg1 was tolerant to various organic solvents at a concentration of 5% (w/v) and also to sodium acetate up to 200 mmol L−1. Xylobiose and xylotriose with a 4-O-methylglucuronic acid branching were the main products of beechwood xylan hydrolysis, and the time course of hydrolysis was not affected by NaCl 0.5 mol L−1 or sea water. To the best of our knowledge, this is the first report of a halotolerant endoxylanase from fungal origin. The properties of Excg1 suggested good potential for use in lignocellulose saccharification processes particularly using sea water or under high salt conditions, or in the presence of residues and/or byproducts of pretreatment steps, contributing to improve the economic viability of 2G ethanol production.
تدمد: 1381-1177
DOI: 10.1016/j.molcatb.2017.05.002
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::101268f088cc3c2746f6e948ff253c1f
https://doi.org/10.1016/j.molcatb.2017.05.002
Rights: CLOSED
رقم الانضمام: edsair.doi...........101268f088cc3c2746f6e948ff253c1f
قاعدة البيانات: OpenAIRE
الوصف
تدمد:13811177
DOI:10.1016/j.molcatb.2017.05.002