Academic Journal

Construction of Ag-modified ZnO/g-C3N4 heterostructure for enhanced photocatalysis performance.

التفاصيل البيبلوغرافية
العنوان: Construction of Ag-modified ZnO/g-C3N4 heterostructure for enhanced photocatalysis performance.
المؤلفون: Liu, Shanshan1 (AUTHOR) liujh@henu.edu.cn, Cheng, Shaoli1 (AUTHOR), Zheng, Jiale1 (AUTHOR), Liu, Junhui1 (AUTHOR) hmingju@163.com, Huang, Mingju1 (AUTHOR)
المصدر: Journal of Chemical Physics. 10/21/2024, Vol. 161 Issue 15, p1-12. 12p.
مصطلحات موضوعية: *FINITE difference time domain method, *SILVER nanoparticles, *DENSITY functional theory, *RHODAMINE B, *RESONANCE effect
مستخلص: ZnO/g-C3N4 heterojunction modified with Ag nanoparticles (ZnO/CN/Ag) was synthesized by depositing ZnO nanorods/Ag nanoparticles onto g-C3N4 nanosheets. Under xenon lamp irradiation, 99% of Rhodamine B (RhB) was degraded by ZnO/CN/Ag-5% composite within 30 min, which was much higher than the degradation efficiency of ZnO and ZnO/CN. The synergistic effect of g-C3N4 and ZnO, along with the localized surface plasmon resonance effect of Ag NPs, contributes to the improvement of photocatalytic performance. Ag nanoparticle provides another charge transfer path from g-C3N4 to ZnO, which speeds up the separation of electron–hole pairs. Meanwhile, the catalyst had good stability and recyclability. Finite-difference time-domain method and the density functional theory were used to obtain the charge transfer process. The photodegradation process has been studied in depth. [ABSTRACT FROM AUTHOR]
قاعدة البيانات: Academic Search Index
الوصف
تدمد:00219606
DOI:10.1063/5.0226195