Pd(0)-Catalyzed Direct Inter- and Intramolecular C–H Functionalization of 4-Carboxyimidazoles
| العنوان: | Pd(0)-Catalyzed Direct Inter- and Intramolecular C–H Functionalization of 4-Carboxyimidazoles |
|---|---|
| المؤلفون: | Virginie Sophie Poncelet, Christophe Hoarau, Antoine Peresson, Thibaut Perse, Steven Frippiat, Christine Baudequin, Olivier Querolle, Cédric Schneider, Vincent Levacher, Patrick Angibaud, Lieven Meerpoel, Yvan Ramondenc, Laurent Bischoff |
| المساهمون: | Chimie Organique et Bioorganique : Réactivité et Analyse (COBRA), Institut Normand de Chimie Moléculaire Médicinale et Macromoléculaire (INC3M), Institut de Chimie du CNRS (INC)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Normandie Université (NU)-Institut national des sciences appliquées Rouen Normandie (INSA Rouen Normandie), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Université Le Havre Normandie (ULH), Normandie Université (NU)-Université de Rouen Normandie (UNIROUEN), Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS)-Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Institut de Chimie du CNRS (INC)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie Organique Fine (IRCOF), Université de Rouen Normandie (UNIROUEN), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS), Janssen Research & Development, Institut de Chimie Organique Fine (IRCOF), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS)-Université de Rouen Normandie (UNIROUEN), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS)-Institut Normand de Chimie Moléculaire Médicinale et Macromoléculaire (INC3M), Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS)-Université de Rouen Normandie (UNIROUEN), Normandie Université (NU)-Université Le Havre Normandie (ULH), Normandie Université (NU)-Institut national des sciences appliquées Rouen Normandie (INSA Rouen Normandie), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS)-Université Le Havre Normandie (ULH), Normandie Université (NU)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS) |
| المصدر: | SYNLETT SYNLETT, Georg Thieme Verlag, 2020, 31 (10), pp.1015-2021. ⟨10.1055/s-0040-1708003⟩ SYNLETT, Georg Thieme Verlag, 2020, 31 (10), pp.1015-1021. ⟨10.1055/s-0040-1708003⟩ |
| بيانات النشر: | HAL CCSD, 2020. |
| سنة النشر: | 2020 |
| مصطلحات موضوعية: | Alkenylation, 010402 general chemistry, Ring (chemistry), 01 natural sciences, Medicinal chemistry, Catalysis, C-H functionalization, imidazole, chemistry.chemical_compound, Imidazole, [CHIM]Chemical Sciences, ComputingMilieux_MISCELLANEOUS, heterocycles, catalysis, [CHIM.ORGA]Chemical Sciences/Organic chemistry, 010405 organic chemistry, Aryl, Organic Chemistry, Arylation, palladium, Palladium catalysis, alkenylation C-H functionalization, 0104 chemical sciences, Solvent, C-H Functionalisation, chemistry, Intramolecular force, alkenation, Surface modification |
| الوصف: | International audience; The palladium-catalyzed arylation and alkenylation of N-substituted methyl imidazole-4-carboxylates are described through inter- and intramolecular pathways. Both direct C2–H and C5–H arylation and alkenylation proceed under Pd(0)/Cu(I) cooperative catalysis and Pd(0) catalysis, respectively, in low-polarity 1,4-dioxane solvent. The methodology gives access to C2 (hetero)aryl or alkenyl imidazoles as well as innovative C2- and C5-arylated fused imidazoles tricycles with a five- to seven-membered middle ring. |
| اللغة: | English |
| تدمد: | 0936-5214 1437-2096 |
| DOI: | 10.1055/s-0040-1708003⟩ |
| URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::c9434a083cc8e00032950a76fb30e594 https://hal-normandie-univ.archives-ouvertes.fr/hal-02548986 |
| Rights: | OPEN |
| رقم الانضمام: | edsair.doi.dedup.....c9434a083cc8e00032950a76fb30e594 |
| قاعدة البيانات: | OpenAIRE |
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|
| IllustrationInfo |