Fluorinated saccharides on the Si(001) surface

التفاصيل البيبلوغرافية
العنوان: Fluorinated saccharides on the Si(001) surface
المؤلفون: Anna Szwajca, Henryk Koroniak, Magdalena Rapp, Monika Bilska, Maciej Krzywiecki
المصدر: Applied Surface Science. 274:221-230
بيانات النشر: Elsevier BV, 2013.
سنة النشر: 2013
مصطلحات موضوعية: Chemistry, Analytical chemistry, General Physics and Astronomy, Infrared spectroscopy, Self-assembled monolayer, Surfaces and Interfaces, General Chemistry, Condensed Matter Physics, Surfaces, Coatings and Films, Contact angle, X-ray photoelectron spectroscopy, Attenuated total reflection, Monolayer, Molecule, Physical chemistry, Wetting
الوصف: The attachment of saccharide molecules directly to silicon surface has been for the first time. Oxygen free silicon surface was functionalized with monosacharides thanks to UV irradiation in acetonitryl solution (254 nm). Selected derivatives of pentofuranose were protected at the C-1 and C-2 position. The remaining hydroxyl group at C-3 or C-5 was suitable for direct attachment to H-terminated Si(0 0 1) surface via Si O C bonds. The binding energy of the saccharide to the Si surface was investigated by quantum mechanical calculations method. The Parametric Method 5 (PM5) calculations confirmed that the formation of Si O C bonds was chemically possible. Synthesis of new fluorinated carbohydrates has been described. The resulting monolayers were characterized by Atomic Force Microscopy (AFM), X-ray photoelectron spectroscopy (XPS) and Attenuated Total Reflection (ATR) infrared spectroscopy. The effect of incorporating fluorine atom or CF3 group into self-assembled monosaccharide monolayers was studied using a water contact angle measurements. The resulting surface wettability of different fluorinated components on one kind of planar substrate enables an answer which of derivative is required for the preparation of the hydrophobic monolayer.
تدمد: 0169-4332
DOI: 10.1016/j.apsusc.2013.03.020
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::d35b306b13fccf0f65a20bcca543cdea
https://doi.org/10.1016/j.apsusc.2013.03.020
رقم الانضمام: edsair.doi...........d35b306b13fccf0f65a20bcca543cdea
قاعدة البيانات: OpenAIRE
الوصف
تدمد:01694332
DOI:10.1016/j.apsusc.2013.03.020